*Result*: A new analytical expression based on the one trap one recombination model to describe thermally assisted optically stimulated luminescence decay curves; simulation results and thermal assistance study.

Title:
A new analytical expression based on the one trap one recombination model to describe thermally assisted optically stimulated luminescence decay curves; simulation results and thermal assistance study.
Authors:
Polymeris GS; RadioCarbon Dating and Other Technologies (RCDOT) Laboratory, Institute of Nanoscience and Nanotechnology, NCSR 'Demokritos', Aghia Paraskevi Attikis, 15341, Greece. Electronic address: g.polymeris@inn.demokritos.gr., Kitis G; Laboratory of Nuclear Physics and Elementary Particles, School of Physics, Aristotle University of Thessaloniki, 54124, Greece.
Source:
Applied radiation and isotopes : including data, instrumentation and methods for use in agriculture, industry and medicine [Appl Radiat Isot] 2025 Dec; Vol. 226, pp. 112107. Date of Electronic Publication: 2025 Aug 14.
Publication Type:
Journal Article
Language:
English
Journal Info:
Publisher: Pergamon Press Country of Publication: England NLM ID: 9306253 Publication Model: Print-Electronic Cited Medium: Internet ISSN: 1872-9800 (Electronic) Linking ISSN: 09698043 NLM ISO Abbreviation: Appl Radiat Isot Subsets: MEDLINE; PubMed not MEDLINE
Imprint Name(s):
Original Publication: Oxford ; New York : Pergamon Press, c1993-
Entry Date(s):
Date Created: 20250823 Latest Revision: 20251111
Update Code:
20260130
DOI:
10.1016/j.apradiso.2025.112107
PMID:
40848358
Database:
MEDLINE

*Further Information*

*Thermally assisted optically stimulated luminescence encompasses simultaneous thermal and optical stimulation, immediately after a thermoluminescence measurement up to 500 °C. While two different measuring modes were proposed, none of these was ever simulated so far. The present work attempts to fill this scientific hiatus by using the one trap one recombination model and Python programming language to generate both linear as well as isothermal TA - OSL decay curves. Analytical expressions using the unique master equation and the appropriate stimulation function were generated. For the case of linear TA - OSL, exploitation of common methods of kinetic analysis such as deconvolution using the Lambert W function, initial rise, various heating rate and peak shape methods is reported towards the calculation of the thermal assistance activation energy. The agreement between numerical and analytical TA - OSL models ensures that despite the fact that all methods work sufficiently, initial rise and deconvolution were proven to be the most reliable and accurate method for evaluating kinetic parameters for the case of linear TA - OSL peaks. For the case of isothermal TA - OSL, a specific protocol that simulates the measurement of this signal at incrementally increasing stimulation temperatures was implemented. The results indicate that calculation is more accurate when optical stimulation is faint. Finally, phototransfer thermoluminescence was studied as a proxy for the presence or absence of re-trapped photoionized electrons.
(Copyright © 2025 Elsevier Ltd. All rights reserved.)*

*Declaration of competing interest The authors declare that they have no known competing financial interests or personal relationships that could have appeared to influence the work reported in this paper.*